Search results for " Dissociation"

showing 10 items of 99 documents

Nature of (C5Me5)2Mo2O5in water–methanol at pH 0–14. On the existence of (C5Me5)MoO2(OH) and (C5Me5)MoO2+: a stopped-flow kinetic analysis

2002

A stopped-flow analysis of compound Cp*2Mo2O5 (Cp* = η5-C5Me5) in 20% MeOH–H2O over the pH range 0–14 has provided the speciation of this molecule as well as the rate and mechanism of interconversion between the various species that are present in solution. The compound is a strong electrolyte in this solvent combination, producing the Cp*MoO2+ and Cp*MoO3− ions in equilibrium with a small amount of Cp*MoO2(OH), the latter attaining ca. 15% relative amount at pH 4. At low pH (  6. The acid dissociation constant of Cp*MoO2(OH) has been measured directly (pK = 3.65 ± 0.02) while the pK for the protonation equilibrium leading to Cp*MoO3H2+ is estimated as  5. The prevalent pathway at high pH i…

010405 organic chemistryStereochemistryChemistryInorganic chemistryKineticsProtonationGeneral Chemistry010402 general chemistry01 natural sciencesCatalysisAcid dissociation constant0104 chemical sciencesCatalysisMetalSolventStrong electrolytevisual_artMaterials Chemistryvisual_art.visual_art_mediumMoleculeNew J. Chem.
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HIV infection with viro-immunological dissociation in a patient with polycystic kidney disease: Candidate for transplantation?

2016

Highlights • Autosomal dominant polycystic kidney disease is the most common among inherited cystic kidney diseases. • Patients with HIV infection are at risk of developing acute kidney injury and chronic kidney disease. • We provide the first report of HIV infection in a patient with polycystic kidney disease. • Lymphopenia should not contraindicate kidney transplantation in patients with HIV infection.

030232 urology & nephrologyHuman immunodeficiency virus (HIV)Case ReportViro-immunological dissociationmedicine.disease_causeVirological response03 medical and health sciences0302 clinical medicinePolycystic kidney diseaseLymphopeniaPolycystic kidney diseaseMedicine030212 general & internal medicineStage (cooking)Kidney transplantationTransplantationurogenital systembusiness.industryHIV; Lymphopenia; Polycystic kidney disease; Transplantation; Viro-immunological dissociation; Infectious Diseasesvirus diseasesHIVmedicine.diseaseAntiretroviral therapyTransplantationInfectious DiseasesImmunologybusinessIDCases
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PERITRAUMATIC FACTORS AND POSTTRAUMATIC SYMPTOMS IN CHILD SEXUAL ABUSE CASES

2017

Health and legal professionals are aware of adverse effects child sexual abuse (CSA) can have on child development as well as the individual differences in severity of psychological outcomes. The objective of this pilot study was to identify possible explanations that could account for the CSA psychological outcome variability and give insights for further research. A sample of 25 Russian speaking girls by the decision of the person directing the proceedings were recognized as CSA victims and were assigned to psychological or complex psychiatric and psychological expert examination. During examination demographical data was collected and several self-report measures regarding peritraumatic …

050103 clinical psychologybusiness.industry05 social sciencesStepwise regression analysisChild developmentPeritraumatic distressPeritraumatic dissociationChild sexual abuseCorrelation analysisMedicine0501 psychology and cognitive sciencesAdverse effectbusiness050104 developmental & child psychologyClinical psychologyVisuomenės sveikata
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Improving Dissolution Behavior and Oral Absorption of Drugs with pH-Dependent Solubility Using pH Modifiers: A Physiologically Realistic Mass Transpo…

2021

Orally dosed drugs must dissolve in the gastrointestinal (GI) tract before being absorbed through the epithelial cell membrane. In vivo drug dissolution depends on the GI tract's physiological conditions such as pH, residence time, luminal buffers, intestinal motility, and transit and drug properties under fed and fasting conditions (Paixao, P. et al. Mol. Pharm. 2018 and Bermejo, et al. M. Mol. Pharm. 2018). The dissolution of an ionizable drug may benefit from manipulating in vivo variables such as the environmental pH using pH-modifying agents incorporated into the dosage form. A successful example is the use of such agents for dissolution enhancement of BCS class IIb (high-permeability,…

Absorption (pharmacology)Chemistry PharmaceuticalAdministration OralBiological AvailabilityPharmaceutical ScienceModels BiologicalDosage formAcid dissociation constantExcipientsFumaratesDrug DiscoveryHumansComputer SimulationDissolution testingSolubilityTartratesDissolutionChromatographyChemistryHydrogen-Ion ConcentrationStomach emptyingBetaineDrug LiberationSolubilityGastrointestinal AbsorptionDrug DesignMolecular MedicineWeak baseMolecular Pharmaceutics
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Psychometric properties of the dissociative symptoms scale (DSS) in Italian outpatients and community adults

2020

This study investigated the psychometric properties of the Dissociative Symptoms Scale (DSS) among Italian adults from outpatient and community samples. The DSS is a self-report measure of clinically relevant dissociation in adults. An Italian translation of the DSS was administered with measures of lifetime traumatic experiences, psychoform dissociation, and somatoform dissociation to 175 psychiatric outpatients and 423 individuals from the community. The DSS scores for outpatient and community adults were significantly different and showed good internal reliability, good convergent and construct validity, and a four-factor structure (depersonalization and derealization, gaps in awareness …

Adult050103 clinical psychologyvalidityDissociation (neuropsychology)Psychometricsmedicine.drug_classDissociative DisordersDissociativeSomatoform dissociation03 medical and health sciences0302 clinical medicineOutpatientsDepersonalizationDerealizationmedicineHumans0501 psychology and cognitive sciencesPsychiatric Status Rating Scalesreliability05 social sciencesReproducibility of ResultsConstruct validityCognitionmedicine.disease030227 psychiatryPsychiatry and Mental healthClinical PsychologyItalymedicine.symptomPsychologydissociative symptoms scaleDissociationClinical psychology
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Qualitative assessment of SARS-CoV-2-specific antibody avidity by lateral flow immunochromatographic IgG/IgM antibody assay.

2020

Abstract Knowledge of the precise timing of SARS‐CoV‐2 infection may be of clinical and epidemiological relevance. The presence of low‐avidity IgGs has conventionally been considered an indicator of recent infection. Here, we carried out qualitative assessment of SARS‐CoV‐2‐specific antibody avidity using an urea (6M) dissociation test performed on a lateral flow immunochromatographic IgG/IgM device. We included a total of 76 serum specimens collected from 57 COVID‐19 patients, of which 39 tested positive for both IgG and IgM and 37 only for IgG. Sera losing IgG reactivity after urea treatment (n = 28) were drawn significantly earlier (P = .04) after onset of symptoms than those which prese…

AdultMaleCoronavirus disease 2019 (COVID-19)Severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2)Short CommunicationAntibody AffinityShort CommunicationsAntibodies ViralImmunoglobulin GSARS‐CoV‐2COVID-19 Serological Testing03 medical and health sciences0302 clinical medicineavidityVirologyurea dissociationMedicineHumansantibodiesIn patientAvidity030212 general & internal medicineQualitative ResearchAgedAged 80 and overImmunoassayCovid‐19medicine.diagnostic_testbiologybusiness.industrySARS-CoV-2COVID-19Middle AgedVirologySpecific antibodyInfectious DiseasesImmunoglobulin MImmunoglobulin MImmunoassayImmunoglobulin GImmunologybiology.protein030211 gastroenterology & hepatologyFemaleAntibodybusinessJournal of medical virology
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Tapping doesn't help: Synchronized self-motion and judgments of musical tempo.

2019

For both musicians and music psychologists, beat rate (BPM) has often been regarded as a transparent measure of musical speed or tempo, yet recent research has shown that tempo is more than just BPM. In a previous study, London, Burger, Thompson, and Toiviainen (Acta Psychologica, 164, 70–80, 2016) presented participants with original as well as “time-stretched” versions of classic R&B songs; time stretching slows down or speeds up a recording without changing its pitch or timbre. In that study we discovered a tempo anchoring effect (TAE): Although relative tempo judgments (original vs. time-stretched versions of the same song) were correct, they were at odds with BPM rates of each stimulus…

AdultMaleLinguistics and LanguageTime FactorsAdolescentMovementAudio time-scale/pitch modificationExperimental and Cognitive PsychologyRhythmMusicalStimulus (physiology)Perception–action dissociation050105 experimental psychologyLanguage and LinguisticsPerceptual sharpeningFingersTime for Action: Reaching for a Better Understanding of the Dynamics of Cognition03 medical and health sciencesJudgmentMotionYoung Adult0302 clinical medicineRhythmSensorimotor synchronizationSelf motionHumans0501 psychology and cognitive sciencesTempo illusion05 social sciencesSensory SystemsAuditory PerceptionTappingFemalePsychologyTimbreBeat (music)030217 neurology & neurosurgeryMusicCognitive psychologyAttention, perceptionpsychophysics
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Capillary electrokinetic fractionation mass spectrometry (CEkF/MS): Technology setup and application to metabolite fractionation from complex samples…

2014

Capillary electrokinetic fractionation (CEkF) is investigated as a new, simple, and robust approach for semipreparative and analytical sample analysis based on pKa -dependant pH-driven electrophoretic mobility. CEkF was optimized with contactless conductivity detection and conducted with 10 kV reverse voltage for 10 min, then coupled on/at-line to ESI/MS. We propose a semi-empirical model with 14 representative compounds based on the correlation between sample/medium pH regulating the partial charge, the electrokinetic loading of the capillary and intensity (I) of analytes. According to the model, an empirical function (I = f (pH)) could be derived to calculate the acid dissociation constan…

AnalyteChromatographySulfur CompoundsChemistryCapillary actionClinical BiochemistryAnalytical chemistryElectrophoresis CapillaryWineFractionationHydrogen-Ion ConcentrationMass spectrometryBiochemistryMass SpectrometryAcid dissociation constantAnalytical ChemistryElectrophoresisElectrokinetic phenomenaModels ChemicalSpectroscopy Fourier Transform InfraredIon cyclotron resonanceELECTROPHORESIS
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Theoretical Determination of the pK a Values of Betalamic Acid Related to the Free Radical Scavenger Capacity: Comparison Between Empirical and Quant…

2015

Health benefits of dietary phytochemicals have been suggested in recent years. Among 1000s of different compounds, Betalains, which occur in vegetables of the Cariophyllalae order (cactus pear fruits and red beet), have been considered because of reducing power and potential to affect redox-modulated cellular processes. The antioxidant power of Betalains is strictly due to the dissociation rate of the acid moieties present in all the molecules of this family of phytochemicals. Experimentally, only the pK a values of betanin were determined. Recently, it was evidenced it was evidenced as the acid dissociation, at different environmental pHs, affects on its electron-donating capacity, and fur…

AntioxidantPyridinesmedicine.medical_treatmentBetalainsHealth Informatics010402 general chemistry01 natural sciencesGeneral Biochemistry Genetics and Molecular BiologyAcid dissociation constantAntioxidantschemistry.chemical_compoundComputational chemistryBetalamic Acid antioxidants pKa predictions empirical methods DFTmedicineOrganic chemistryA valueMoleculeBetaninQuantum chemical010405 organic chemistryFree Radical ScavengersFree radical scavengerSettore CHIM/08 - Chimica Farmaceutica0104 chemical sciencesComputer Science ApplicationschemistryModels ChemicalBetalamic acid
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Masstodon : a tool for assigning peaks and modeling electron transfer reactions in top-down mass spectrometry

2019

Abstract: Top-down mass spectrometry methods are becoming continuously more popular in the effort to describe the proteome. They rely on the fragmentation of intact protein ions inside the mass spectrometer. Among the existing fragmentation methods, electron transfer dissociation is known for its precision and wide coverage of different cleavage sites. However, several side reactions can occur under electron transfer dissociation (ETD) conditions, including nondissociative electron transfer and proton transfer reaction. Evaluating their extent can provide more insight into reaction kinetics as well as instrument operation. Furthermore, preferential formation of certain reaction products can…

Apolipoprotein A-IUbiquitinChemistry010401 analytical chemistryElectronsSubstance PTracing010402 general chemistryMass spectrometry01 natural sciencesMass Spectrometry0104 chemical sciencesAnalytical ChemistryIonElectron-transfer dissociationChemical kineticsElectron transferChemistryFragmentation (mass spectrometry)Chemical physicsMass spectrumAlgorithmsSoftwareAnalytical chemistry
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